Open iTunes by clicking on the desktop icon. Select the "Summary" tab in the main iTunes browser.
Select "Manually Manage Music and Videos" from the list of options. This will disable the auto sync program and allow you to access the iPod independent of the iTunes music program.
Click on the "iPod" icon on your desktop and highlight any music or media in the library you wish to delete.
The ability to store large amounts of music and video is what makes the iPod one of the most popular portable media devices on the market today. But even if you own one with a lot of memory, it is still possible to run out of space. So if you have filled your iPod to the brim with media but still want to add more, you are going to have to make a little room. Deleting the content on your iPod is a pretty straightforward process that will allow you to better manage your music and media library.
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