Click "Apple TV" in the iTunes side window to access your Apple TV, and click "File" at the top of iTunes. Click "Transfer Purchases from Apple TV."
Insert the dock connector cable into your iPod, and plug the other end in the USB port on your computer.
Click the "iPod" tab in the iTunes side window, and click "Movies" in the iPod's synchronization window in iTunes. Click "Sync Movies" and click the movie you want to transfer to the iPod.
Purchased iTunes movies stored on your Apple TV can be transferred to any Apple mobile device, including your iPod, through iTunes' media synchronization. When iTunes connects to your Apple TV, all purchased content is copied from the Apple TV and stored in iTunes. Once transferred, movies can then be synced to your iPod for portable playback. According to Apple, only purchased movies can be transferred from your Apple TV to alternate devices due to the restrictions on rental movies.
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